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Reference Number UKRI1107
Title Stabilising superconductivity in thin film nickelates
Status Started
Energy Categories Energy Efficiency 20%;
Not Energy Related 70%;
Other Power and Storage Technologies (Energy storage) 10%;
Research Types Basic and strategic applied research 100%
Science and Technology Fields PHYSICAL SCIENCES AND MATHEMATICS (Physics) 50%;
PHYSICAL SCIENCES AND MATHEMATICS (Metallurgy and Materials) 50%;
UKERC Cross Cutting Characterisation Not Cross-cutting 100%
Principal Investigator Peter Wahl
University of St Andrews
Award Type Standard
Funding Source EPSRC
Start Date 01 October 2025
End Date 01 April 2029
Duration 42 months
Total Grant Value £1,434,808
Industrial Sectors Unknown
Region Scotland
Programme NC : Physical Sciences
 
Investigators Principal Investigator Peter Wahl , University of St Andrews
  Other Investigator Phil King , University of St Andrews
Andreas Rost , University of St Andrews
Web Site
Objectives
Abstract Developing more energy-efficient technologies is a key component of sustainable economic growth. Superconductors can make a key contribution to such technologies, however their ground state is typically only reached at very low temperatures. Only one group of materials, the cuprate high-temperature superconductors, so far exhibits superconductivity at temperatures above the boiling point of liquid nitrogen and at ambient pressure, which has made it challenging to develop a universal understanding of the pairing mechanism in these materials. Recently, superconductivity at similarly high temperatures has been reported in a second class of transition metal oxides, the lanthanum nickelates, albeit so far only under pressure. Discovery of a second class of transition metal oxides that exhibits high temperature superconductivity promises new opportunities to establish an understanding of the pairing mechanism in these materials and vastly better possibilities their properties in applications. The lanthanum nickelates are structurally very similar to the cuprates: they are both perovskite oxides, and superconductivity is observed in layered compounds of the Ruddlesden-Popper (RP) series – suggesting that similar physics might be at play. The primary objective of this research proposal is to systematically investigate the ground states of RP type phases derived from lanthanum nickelates in a quest to stabilise the superconductivity at ambient pressure as well as establish their correlated phases and understand their origin. To be able to harvest this potential high temperature superconductivity, but also improve our understanding of and ability to design correlated phases in transition metal oxides, we propose here an approach that combines thin film growth with characterisation by spectroscopies and electronic transport and ab-initio modelling to identify the key physics, enable identification of the superconducting phase, and unravel the mystery of high-temperature superconductivity in lanthanum nickelates. To achieve this objective, we will Use advanced spectroscopic methods to understand the electronic structure and correlated phases of single crystals of lanthanum nickelates Establish growth of electronic designer metamaterials, consisting of layered structures of different members of the Ruddlesden-Popper series of the lanthanum nickelates Employ a range of methods to identify the superconducting phase and stabilise it in thin films at ambient pressur
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Added to Database 07/01/26